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GPU mining is the way to go, as at August 2011, until something better arrives on the market. There are plenty of GPUs out there, but only a handful offer the best performance when comparing total number of Bitcoins generated vs. power consumed vs. initial purchase cost of the chip.
Which GPUs provide the best performance in regards to Bitcoin Generation vs. Power Consumption?
This question may no longer be relevant as acquiring GPUs for mining purposes is no longer seen as being a good business decision. – Stephen Gornick – 2013-03-27T12:23:30.840
@StephenGornick: Even still, it's an old question that was valid in 2011. There is no need to down vote it. Just post a new answer stating the change in the network. Such answers are acceptable on StackExchange because many questions can have differing answers as they age. Post an answer and remove the down-vote and I'll give you the check. – RLH – 2013-03-28T10:22:03.233
FYI, I've posted this question with the intent that it can become a Community Wiki. This is a question with a dynamic answer. – RLH – 2011-08-30T21:15:28.063